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Additional info for Comprehensive Natural Products II: Chemistry and Biology: Natural Products Structural Diversity-I Secondary Metabolites Organization and Biosynthesis
28 Unsaturated Fatty Acids Scheme 13 Putatative biosynthetic pathway of cyclopropenyl fatty acids. 5 Summary and Future Prospects The invention and application of novel mechanistic probes (deutero-, fluoro-, thia-containing substrate analogues) has led to a more sophisticated understanding of how fatty acid desaturases and related enzymes carry out their ultra-selective oxidation chemistry. Three mechanistic issues with respect to desaturase mechanism have been addressed with varying levels of success.
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Soc. 1999, 121, 3897. 7. I. Feussner; C. Wasternack, Annu. Rev. Plant Biol. 2002, 53, 275. 8. W. L. Smith; R. C. Murphy; D. E. Vance; J. E. , Biochemistry of Lipids, Lipoproteins and Membranes, 4th ed; Elsevier: Amsterdam, 2002; pp 341–371. 9. J. M. Dyer; S. Stymne; A. G. Green; A. S. Carlsson, Plant J. 2008, 54, 640. 10. J. A. Napier, Annu Rev. Plant. Biol. 2007, 58, 295. 11. A. Dobrzyn; J. M. Ntambi, Prostaglandins Leukot. Essent. Fatty Acids 2005, 73, 35. 12. B. Phetsuksiri; M. Jackson; H. Scherman; M.
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