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Chem. Solids 35 (1974) 657. BonnelIe, C, Karnatak, R. : Chem. Phys. Letters 14 (1972) 145. , Siegmann, H. : Phys. Letters 24A (1967) 733. : J. Phys. Chem. Solids 36 (1975) 575. : These CNAM, Paris, 1975. : J. de Phys. 35 (1974) 295. : under preparation. , Lachere, G. : 5th International Conference on Plutonium and Other Actinides, 31. 32. 33. 34. 35. : under preparation. : J. Chem. Phys. 57(1972) 899. , Werme, L. : J. Phys. B8 (1975) L18. Larson, D. , Adams, R. : Surface Science 47 (1975) 413. : 5th International Conference on Plutonium and Other 17.

This is in agreement with the suggestion by Friedel (36) according to which the 5 f electrons are appreciably more localized about each ion in the high-temperature phases than in monoclinic a - P u . Our results confirm that the expansion in the atomic volume of the 6-phase with respect to the a-phase (see Fig. 8) is associated with an increase in the number of localized electrons forming a screen to the nuclear charge. The same modifications are likely in the intermetallic compounds where an increase in the Pu interatomic distance is stabilized, for example, by the introduction of small quantities of trivalent elements (37).

21. 22. 23. 24. 25. North-Holland Amsterdam 1976. Actinides, North-Holland, Amsterdam 1976. 36. : Rapport CEA n ° 766 (1958) Paris. 37. , J of Nuclear Materials 39 (1971) 350. 38. Tucker, T. , Nestor, C. : Phys. Rev. 174 (1968) 118. 39. : Solid State Comm. 9 (1971) 1369. 40. , Freeman, A. : Phys. Rev. B 7 (1973) 4454. 41. : J. Physique 33 (1972) C3-57. 42. : Phys. Rev. B6 (1972) 2139. 43. , Maneseu, L: C. R. Paris 267B (1968) 817. 44. R. Paris 256 (1963) 112 and 257 (1963) 2980. 47 C. Bonnelle 45.

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